Case Studies, Metals and Glass
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The Research Group

  • ARPA-E funded project
  • PNNL, U. of North Texas, Citrine Informatics

Award# DE-AR0001613
ONWARDS, PM Bob Ledoux

ARPA-E
Pacific Northwest National Laboratory
University of North Texas
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The Problem

  • Current nuclear waste storage is too expensive
  • Waste forms are space-inefficient and prone to hazardous leaching, mechanical failure, and thermal degradation
  • Design novel waste form with improvements in five performance metrics
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The Process

  • Built database of nuclear waste form materials properties for model waste stream
  • Developed ML models to predict strength, chemical durability, phase stability, vitrification
  • Optimized nuclear waste glass for waste loading, strength, chemical durability, thermal stability
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The Outcome

  • >2x waste loading
  • 20x reduction in waste volume
  • >2x mechanical strength
  • Multi-objective design workflow
Likelihood of improvement score
E1, E2 = Promising candidates predicted by ML

Hegde et al. Digit. Discov. (2024);    Allec et al. J. Am. Ceram. Soc. (2024);    Du et al. Trans. Am. Nucl. Soc. (2024);    Kalahe et al. J. Nucl. Mat. (2024)